By Richard J. Pankhurst
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Additional resources for Biological identification: The principles and practice of identification methods in biology
8) −E at each base pair n on the π stack. 9) for k = 1, 2, . . , L. 4) splits into two cosine bands such that E ∈ −t − 2 t2 + 2t↑ , −t + t2 + 2t↑ 2 ∪ t− 2 t2 + 2t↑ , t + t2 + 2t↑ 2 . 74 eV are being used. Therefore, we will assume tqi = 2ti and set the energy scale by ti ≡ 1 for hopping between GC pairs. Furthermore, since the energetic diﬀerences in the adiabatic electron aﬃnities of the bases are small , we choose εi = 0 for all i. The physics of the ﬁshbone model was ﬁrst discussed for poly(G)-poly(C) in .
D. A. A. Ratner and L. D. A. Siebbeles, J. Am. Chem. Soc. 127, 14894 (2005). 31. K. C. Grozema, C. M. A. Siebbeles, J. Am. Chem. Soc.
This discrepancy is not surprising since the charge transfer rates will be aﬀected by the Coulomb interaction between the Sa−• anion and the hole generated in the system. 3. 2 Charge Transfer Through DNA 37 Fig. 8. Survival probability for sequences 4a–4d as a function of time in absence (top) and in presence (bottom) of the Coulomb potential of Sa•− the nucleobases. The survival probabilities calculated in the case, where the Coulomb interaction is included in the calculations, are shown in Fig.